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By Lars Onsager (auth.), Stephan L. Mintz, Susan M. Widmayer (eds.)
leagues and, in lots of situations, scholars, of Professor Onsager. Professor Onsager, himself, has contributed a paper on Illife in early occasions" to the quantity. one of the subject matters mentioned are a few attention-grabbing purposes of low temperature experimental thoughts to cardiology and astrophysics. we wish to specific our specific appreciation to Mrs. Helga Billings and leave out Sara Lesser for his or her first-class typing of those lawsuits and to Mrs. Jacquelyn Zagursky, in addition to to Mrs. Billings and leave out Lesser for his or her precious information with the main points of the convention and the ebook of those lawsuits. The Editors CONTENTS part One BIOLOGY existence within the Early Days Lars Onsager. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 The Fluctuating Enzyme Giorgio Careri. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 15 Diffusion keep an eye on in Biochemical Reactions Manfred Eigen. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 37 section Transitions of Phospholipids Julian Sturtevant. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . sixty three conception and Density Measurements of the Lipid Bilayer section Transition John F. Nagle. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . eighty five balance of Helical Nucleic Acids Neville R. Kallenbach. . . . . . . . . . . . . . . . . . . . . . . . . . . ninety five Thermodynamic views and the foundation of existence Sidney W. Fox. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 119 part STATISTICAL MECHANICS excessive Frequency Dielectric reaction in Dipolar structures Roberto Lobo, John E. Robinson, Sergio Rodriguez. 143 ix x CONTENTS distinct Derivation of the Onsager proscribing legislations Thomas J. Murphy 157 The impression of Wall cost at the Capillary upward push of Electrolytes Lars Onsager, Edmund Drauglis 167 Density of States of Topologically Disordered Amorphous Semiconductors Jill C. Bonner, J. F. Nagle 201 Irreversibility Willis E. Lamb, Jr. 213 floor particular warmth of Crystals.
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Extra resources for Quantum Statistical Mechanics in the Natural Sciences: A Volume Dedicated to Lars Onsager on the Occasion of his Seventieth Birthday
Example text
8. F. H. Westheimer~ Advan. Enzymo1. ~~ 455 (1962). 9. W. P. Jencks and M. I~ Page~ Proc. 8th FEBS Meeting~ Amsterdam (1971). 10. G. Careri~ V. Mazzacurati~ M. Sampo1i~ G. Signorelli and P. Fase11a~ Bioch. Bioph. Acta 310~ 305 (1973). 11. M. V. Vo1kenstein~ J. Theor. Biol. ~~ 193 (1972). 12. F. Osawa~ J. Theor. Biol. 39~ 373 (1973). 13. J. M. Schurr~ J. Chem. Phys. ll~ 2820 (1969). 14. M. Hussey and P. Edmonds~ J. Phys. Chem. lL~ 4012 (1971). 15. R. D. White and L. J. Slutsky~ J. Co11. and Interface Sci.
A specific example, again the case of lysozyme, is considered below. A glance to a map showing the lysozyme with its substrate 5 reveals that the acidic and basic side chains that ionize on contact with water are all on the surface of the molecule (and this is the case of Asp 101), with the only exception of the residues Glu 35 and Asp 52 which are very close to the active site. Each of these two residues is connected to a massive section of the macromolecule where the polypeptide chain is highly organized as a kind of helix and pleated sheet.
8 k r- ----- I :........ l : ______I RAB I '- encounter complex 23 ~ ~ k 32 C • (1) reaction product (s) In this scheme the rate constants signify k k k k 12 2l 23 32 the diffusional encounter the diffusional separation the reactive association (trans forma t ion) the reactive dissociation (trans formation) In order to decide whether a reaction is diffusion controlled we have to inspect the relative magnitudes of the rate parameters k and k . e. if the reactive association proceeds DIFFUSION CONTROL IN BIOCHEMICAL REACTIONS 39 fast with respect to the diffusional separation, yielding: Various expressions for the rate constant k , based on 12 phenomenological theory of diffusion, have been derived.