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By Barus C.
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Extra info for The Torsional Magnetic Energy Absorption of an Iron Conductor
Sample text
Hence, both 115 and M! are positive. 1 where the nuclear coordinate Q in the abscissa refers to the breathin g vibration ofthe coordination sphere. At low temperatures, below T , the enthalp y factor c domina tes; I1G is positive and the LS species is the most stable. At high temperatures, above Tc , the entropy factor dominates. I1G is negative and the HS species is the most stable. 1 we have drawn a crossing between the LS and HS curves due to the fact that these states do not have the same symmetry.
72 MOLECULAR MAGNETISM LOW-SPIN-HIGH-SPIN TRANSITION 73 separated in energy from the first excited states. 3. Other interesting examples of spin transition in iron(III) chemistry have been reported by Hendrickson et al. 13. Molecular structure of a tris(dithiocarbamato)iron(I1I) compound Fe(S2 CNR zh (from ref. 37]). A rationalization of the role of solvent molecules has been proposed in the case of tris(4-morpholinecarbodithioato)iron(lII) compounds with the following ligand: 1 \ "fS a N-C "--!
In most cases the orbital degeneracy in a strictly octahedral environment is totally removed by the symmetry lowering. If so, XT is constant in the temperature range where all the molecules are in the same spin state, with (xTks and (XT)HS values, respectively. 1) ~ny other technique that provides different respons es according to whether the state IS LS or HS may also be used to determine the high-spin molar fraction x. Distinct signa~s are obtained in principle when the spin flipping frequency is slower than the techmque ~requenc~.